Second virial coefficients of normal alkanes, linear 1-alkanols (and water), alkyl ethers, and their mixtures

Tsonopoulos, C; Dymond, JH

HERO ID

1186930

Reference Type

Journal Article

Year

1997

Language

English

HERO ID 1186930
In Press No
Year 1997
Title Second virial coefficients of normal alkanes, linear 1-alkanols (and water), alkyl ethers, and their mixtures
Authors Tsonopoulos, C; Dymond, JH
Journal Fluid Phase Equilibria
Volume 133
Issue 1-2
Page Numbers 11-34
Abstract Earlier recommendations [J.H. Dymond et al., Fluid Phase Equilibria 27 (1986) 1-13; C. Tsonopoulos et al., Pure Al. Chem. 61 (1989) 1387-1394.] are updated for C-4-C-8 alkanes and C-1-C-4 alkanols, and more recent values are presented for 1-hexanol. New recommendations are made for butane, on the basis of recent isochoric Burnett measurements. Preliminary recommendations are given for dimethyl, diethyl, and diisopropyl ethers, but nothing definitive can be said about other alkyl ethers due to the limited quantity and quality of the available data. Calculations with a correlation [C. Tsonopoulos, AIChE J. 20 (1974) 263-272] reexamine the dependence of the parameter b of alkanols and parameter a of alkyl ethers on their reduced dipole moment. Also included is the recent [C. Tsonopoulos and J.L. Heidman, Fluid Phase Equilibria 57 (1990) 261-276] analysis of the data for water and water/alkane binaries, along with new analyses of data for the binaries of water with methanol and ethanol. Only other relevant binary data that could be located were for n-hexane/ethanol and methanol/diethyl ether. Recommendations are given for the characteristic binary constant k(ij) for all binaries of interest. In addition, recent results are provided for the critical properties of the industrially important alkyl ethers MTBE, ETBE, TAME, and TAEE, together with recommendations for calculating their B with the 1974 correlation. (C) 1997 Elsevier Science B.V.
Doi 10.1016/S0378-3812(97)00058-7
Wosid WOS:A1997XH67700003
Is Certified Translation No
Dupe Override No
Conference Name 2nd International Workshop on Vapour-Liquid Equilibria and Related Properties in Binary and Ternary Mixtures of Ethers, Alkanes and Alkanols
Conference Date JUL 03-05, 1996
Comments Source: Web of Science A1997XH67700003Scopus URL: https://www.scopus.com/inward/record.uri?eid=2-s2.0-0031165104&doi=10.1016%2fs0378-3812%2897%2900058-7&partnerID=40&md5=58f91710e9be69ac7a09090d66f55c4f
Is Public Yes
Language Text English
Keyword equation of state; method of calculation; second virial coefficient; alkanes; alkanols; alkyl ethers