Increasing atmospheric burden of ethanol in the United States

de Gouw, JA; Gilman, JB; Borbon, A; Warneke, C; Kuster, WC; Goldan, PD; Holloway, JS; Peischl, J; Ryerson, TB; Parrish, DD; Gentner, DR; Goldstein, AH; Harley, RA

HERO ID

1450443

Reference Type

Journal Article

Year

2012

Language

English

HERO ID 1450443
In Press No
Year 2012
Title Increasing atmospheric burden of ethanol in the United States
Authors de Gouw, JA; Gilman, JB; Borbon, A; Warneke, C; Kuster, WC; Goldan, PD; Holloway, JS; Peischl, J; Ryerson, TB; Parrish, DD; Gentner, DR; Goldstein, AH; Harley, RA
Journal Geophysical Research Letters
Volume 39
Issue 15 (2012)
Page Numbers n/a
Abstract The use of ethanol as a transportation fuel in the U.S. increased significantly from 20002009, and in 2010 nearly all gasoline contained 10% ethanol. In accordance with this increased use, atmospheric measurements of volatile organic compounds in Los Angeles in 2010 were significantly enriched in ethanol compared to measurements in urban outflow in the Northeast U.S. in 2002 and 2004. Mixing ratios of acetaldehyde, an atmospheric oxidation product of ethanol, decreased between 2002 and 2010 in Los Angeles. Previous work has suggested that large-scale use of ethanol may have detrimental effects on air quality. While we see no evidence for this in the U.S., our study indicates that ethanol has become a ubiquitous compound in urban air and that better measurements are required to monitor its increase and effects.
Doi 10.1029/2012GL052109
Wosid WOS:000307474900001
Url http://doi.wiley.com/10.1029/2012GL052109
Is Certified Translation No
Dupe Override No
Is Public Yes
Language Text English
Keyword Troposphere; Atmospheric sciences; Air pollution