Characterisation and application of polyurethane copolymers grafted with photoluminescent dyes

Chung, YC; Yang, K; Choi, J; Chun, BC

HERO ID

3575420

Reference Type

Journal Article

Year

2014

Language

English

HERO ID 3575420
In Press No
Year 2014
Title Characterisation and application of polyurethane copolymers grafted with photoluminescent dyes
Authors Chung, YC; Yang, K; Choi, J; Chun, BC
Journal Coloration Technology
Volume 130
Issue 4
Page Numbers 305-313
Abstract Photoluminescent dyes (aminofluorene, naphthalimide, naphtholbenzein, or phenosafranine) were grafted to polyurethane using an allophanate linkage. The photoluminescence properties and the shape recovery effects of polyurethane samples were investigated. The polyurethane was composed of 4,4'-methylenebis (phenylisocyanate), poly(tetramethyleneglycol), and 1,4-butanediol. The dyes were linked through an extra 4,4'-methylenebis(phenylisocyanate) and the carbamate moiety of the polyurethane chains. Polyurethanes with various dye contents were characterised, and the shape recovery and photoluminescence properties were compared. In the case of the tensile mechanical properties, the highest maximum stress was 56 MPa, and the strain remained > 1500% for the entire series. The shape recovery improved as the test cycle was repeated, with up to 100% recovery being achieved, but shape retention decreased as the dye content increased. Finally, the photoluminescence of the polyurethanes was demonstrated by a luminescent light-emission test, together with pH indication capability and the preparation of non-woven fibre using the electrospinning method.
Doi 10.1111/cote.12097
Wosid WOS:000340385400009
Is Certified Translation No
Dupe Override No
Comments Scopus URL: https://www.scopus.com/inward/record.uri?eid=2-s2.0-84904997430&doi=10.1111%2fcote.12097&partnerID=40&md5=794fc3232175e323bfa6090ac1265361
Is Public Yes
Language Text English
Keyword Grafting (chemical); Photoluminescence; Shape optimization; Strain; 1 ,4-Butanediol; Electrospinning method; Maximum stress; Phenylisocyanate; Photoluminescence properties; Photoluminescent dyes; Shape retention; Tensile mechanical properties; Polyurethanes