Simultaneous determination of ascorbic acid and dopamine at electro polymerized manganese (III)-5-[o-(1-imidazolyl)butoxy]phenyl-10,15,20-triphenyl porphrine chloride film modified glassy carbon electrode

Deng Xuerong; Wang Lishi; Zhang Shuifeng; Liu Xiaoxiao; Mo Jinyuan

HERO ID

4854484

Reference Type

Journal Article

Year

2006

HERO ID 4854484
In Press No
Year 2006
Title Simultaneous determination of ascorbic acid and dopamine at electro polymerized manganese (III)-5-[o-(1-imidazolyl)butoxy]phenyl-10,15,20-triphenyl porphrine chloride film modified glassy carbon electrode
Authors Deng Xuerong; Wang Lishi; Zhang Shuifeng; Liu Xiaoxiao; Mo Jinyuan
Journal Chinese Journal of Analytical Chemistry / Fen Xi Hua Xue
Volume 34
Issue 5
Page Numbers 637-641
Abstract The electropolymerization of manganese(III)-5-[o-(1-imidazolyl) butoxyl] phenyl-10, 15, 20-triphenylporphrine chloride (o-ImBPTPPMn (III) Cl) produces stable and electrochemically active film from strong acidic aqueous solutions. Cyclic voltammetry was used to study the in situ growth of poly(o-ImBPTPP Mn (III) Cl) films. The electrode was also employed to study the electrocatalytic oxidation of ascorbic acid (AA) and dopamine (DA), using cyclic voltammery. It has been found that the oxidation of AA at the surface of poly(o-ImBPTPP Mn (III) CI) films modified glassy carbon electrode occurs at a potential of about 407 mV more negative than. that of an unmodified glassy carbon electrode. Differential pulse voltammograms (DPV) of simultaneous determination of AA and DA exhibit linear dynamic rang from 2.0 x 10(-6) to 1.0 x 10(-4) mol/L and a detection limit of 1.0 mu mol/L for AA, and corresponding linear dynamic rang from 6.5 x 10(-7) to 2.6 x 10(-5) mol/L and a detection limit of 0.39 mu mol/l, for DA. In DPV, the poly (o-ImBPFPP Mn (III) Cl) films modified glassy carbon electrode could separate completely the oxidation peak potentials of AA and DA for about 240 mV present in the same buffer solution of 0.1 mol/L phosphate, though at the unmodified glassy carbon electrode the peak potentials were indistinguishable. This modified electrode was quite effective not only to detect AA and DA individually, but also to determine simultaneously each component concentration in the mixture, and they will not affect each other.
Doi 10.1016/S1872-2040(06)60034-0
Wosid WOS:000241620500011
Is Certified Translation No
Dupe Override No
Is Public Yes
Keyword film modified electrode; manganese (III)-5-[o-(1-imidazolyl)butoxy]phenyl-10,15,20-triphenylporphrine chloride; electropolymerization; glassy carbon electrode; ascorbic acid; dopamine