CORRELATIONS BETWEEN RADICAL DISTRIBUTIONS AND STRUCTURAL DEFECTS OF SQUALANE AND POLY(METHYL METHACRYLATE) GLASSES IN THE OXIDATION-KINETICS OF RADICALS

Vasenkov, SV; Bagryansky, VA; Korolev, VV; Tolkatchev, VA

HERO ID

4972307

Reference Type

Journal Article

Year

1991

Language

English

HERO ID 4972307
In Press No
Year 1991
Title CORRELATIONS BETWEEN RADICAL DISTRIBUTIONS AND STRUCTURAL DEFECTS OF SQUALANE AND POLY(METHYL METHACRYLATE) GLASSES IN THE OXIDATION-KINETICS OF RADICALS
Authors Vasenkov, SV; Bagryansky, VA; Korolev, VV; Tolkatchev, VA
Journal Radiation Physics and Chemistry
Volume 38
Issue 2
Page Numbers 191-197
Abstract The kinetics have been studied for two processes whose limiting stage is the diffusion of molecular oxygen: (i) oxidation of radicals after irradiation; and (ii) quenching of phenanthrene phosphorescence. The processes were studied in glassy squalane and poly(methyl methacrylate) matrices. Comparison between the kinetic properties of these processes allowed us to conclude about predominant stabilization of radicals near structural defects of glass. In squalane this manifests itself in anomalously high value of reaction radius for oxidation of radicals and in poly(methyl methacrylate) in quantitative difference in the parameters of distribution in rate constants for processes (i) and (ii).
Doi 10.1016/1359-0197(91)90226-R
Wosid WOS:A1991FX75000010
Is Certified Translation No
Dupe Override No
Comments Scopus URL: https://www.scopus.com/inward/record.uri?eid=2-s2.0-50749134807&doi=10.1016%2f1359-0197%2891%2990226-R&partnerID=40&md5=1301a13328d5646925485ce88d020865
Is Public Yes
Language Text English