Application of chemometrics to the screening of hazardous substances: Part II: Advances in the multivariate characterization and reactivity modelling of haloalkanes

Chiorboli, C; Piazza, R; Carassiti, V; Passerini, L; Tosato, ML

HERO ID

660795

Reference Type

Journal Article

Year

1993

Language

English

HERO ID 660795
In Press No
Year 1993
Title Application of chemometrics to the screening of hazardous substances: Part II: Advances in the multivariate characterization and reactivity modelling of haloalkanes
Authors Chiorboli, C; Piazza, R; Carassiti, V; Passerini, L; Tosato, ML
Journal Chemometrics and Intelligent Laboratory Systems
Volume 19
Issue 3
Page Numbers 331-336
Abstract BIOSIS COPYRIGHT: BIOL ABS. This paper updates a quantitative structure-activity relationship presented previously, where the rate constant of the gas-phase reaction between hydroxyl radical and haloalkanes, k(OH), was related to six atom-counting variables. Five new, group-counting variables have been included in the structural parametrization; they describe the variations in the substitution pattern at the reaction centers (the C-H groups in the molecules). The updated model, contrary to the original, permits one to distinguish between isomeric structures, and is applicable to the previous outliers group of the CH3-C(X)3 (X = halogen) structures. It shows a remarkable predictive capability for few compounds ('external' Q2 = 0.86) over the examined X and Y ranges of the series, and works with descriptors which can be drawn directly from the structures.
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Comments Journal: CHEMOMETRICS INTELLIGENT LAB SYST ISSN:
Is Public Yes
Language Text English
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